Direct Observation of Ultrafast Exciton Formation in a Monolayer of WSe2

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Direct Observation of Ultrafast Exciton Formation in a Monolayer of WSe2.

Many of the fundamental optical and electronic properties of atomically thin transition metal dichalcogenides are dominated by strong Coulomb interactions between electrons and holes, forming tightly bound atom-like states called excitons. Here, we directly trace the ultrafast formation of excitons by monitoring the absolute densities of bound and unbound electron-hole pairs in single monolayer...

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Excitons, Coulomb bound electron-hole pairs, are composite bosons and their interactions in traditional semiconductors lead to condensation and light amplification. The much stronger Coulomb interaction in transition metal dichalcogenides such as WSe2 monolayers combined with the presence of the valley degree of freedom is expected to provide new opportunities for controlling excitonic effects....

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ژورنال

عنوان ژورنال: Nano Letters

سال: 2017

ISSN: 1530-6984,1530-6992

DOI: 10.1021/acs.nanolett.6b04422